Fractal atomic-level percolation in metallic glasses

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Authors

Chen, David Z.
Shi, Crystal Y.
An, Qi
Zeng, Qiaoshi
Mao, Wendy L.
Goddard III, William A.
Greer, Julia R.

Issue Date

2015

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Abstract

Metallic glasses are metallic alloys that exhibit exotic material properties. They may have fractal structures at the atomic level, but a physical mechanism for their organization without ordering has not been identified. We demonstrated a crossover between fractal short-range (<2 atomic diameters) and homogeneous long-range structures using in situ x-ray diffraction, tomography, and molecular dynamics simulations. A specific class of fractal, the percolation cluster, explains the structural details for several metallic-glass compositions. We postulate that atoms percolate in the liquid phase and that the percolating cluster becomes rigid at the glass transition temperature.

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American Association for the Advancement of Science

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In Copyright

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ISSN

0036-8075

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